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环境介质中多溴联苯醚(PBDEs)分布特征的研究进展

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王森, 袁琪, 韩瑞霞, 钱亚利, 丁柳屹. 环境介质中多溴联苯醚(PBDEs)分布特征的研究进展[J]. 环境化学, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
引用本文: 王森, 袁琪, 韩瑞霞, 钱亚利, 丁柳屹. 环境介质中多溴联苯醚(PBDEs)分布特征的研究进展[J]. 环境化学, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
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WANG Sen, YUAN Qi, HAN Ruixia, QIAN Yali, DING Liuyi. Distribution of polybrominated diphenyl ethers (PBDEs) in the environment: A review[J]. Environmental Chemistry, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
Citation: WANG Sen, YUAN Qi, HAN Ruixia, QIAN Yali, DING Liuyi. Distribution of polybrominated diphenyl ethers (PBDEs) in the environment: A review[J]. Environmental Chemistry, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
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环境介质中多溴联苯醚(PBDEs)分布特征的研究进展

  • 1.

    西北大学城市与环境学院, 西安, 710127;

  • 2.

    中国科学院生态环境研究中心环境化学与生态毒理学国家重点实验室, 北京, 100085

  • 基金项目:

    国家自然科学基金（41303073），陕西省青年科技新星计划（2016KJXX-83），陕西省自然科学基础研究计划青年人才项目（2015JQ4101），陕西省教育厅科学研究项目（14JK1731）和西北大学"优秀青年学术骨干支持计划"资助.

Distribution of polybrominated diphenyl ethers (PBDEs) in the environment: A review

  • 1.

    Department of Environmental Sciences, College of Urban and Environmental Sciences, Northwest University, Xi'an, 710127, China;

  • 2.

    State Key Laboratory of Environmental Chemistry and Ecotoxicology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China

  • Fund Project: Supported by the National Natural Science Foundation of China Young Scientist Funds(41303073),Shaanxi Province Youth Science and Technology New Star Plan(2016KJXX-83),Young Talent Project of Natural Science Basic Research Plan in Shaanxi Province of China(2015JQ4101),Scientific Research Project of Shaanxi Provincial Department of Education(14JK1731)and Outstanding Youth Academic Backbone Support Program of Northwest University.

  • 摘要: 由多溴联苯醚（PBDEs）所引起的环境问题越来越受到社会各界的关注，了解环境介质中PBDEs的分布特征是对其污染进行有效控制的前提.本文从非生物介质（大气、水体、沉积物、污泥及土壤）和生物体内（植物、动物、人体及食物链）两方面入手，对PBDEs在世界各地不同环境介质的分布特征进行综述.高溴代PBDEs因其较低的挥发性和水溶性，极易吸附于土壤、底泥和空气悬浮颗粒等固体介质，而低溴代PBDEs在各环境介质中都有检出；生物体中PBDEs的分布特征与生物种类、污染源、营养级以及个体组织的特异性有一定关系，人体血液、母乳、头发等也检出了PBDEs.随着北美、欧盟等地区从2004年开始逐渐对五溴、八溴和十溴PBDEs实施禁用，其含量在北美和欧盟部分地区有所下降，但是由于十溴PBDEs仍在全球很多地区使用，又因其具有持久性和长距离迁移性，要实现环境介质中PBDEs含量的控制仍需要一定时间，因此未来研究仍需对PBDEs生产和使用区域开展污染水平及趋势相关研究，并对PBDEs的环境行为深入探讨.
    Abstract: Environmental problems induced by polybrominated diphenyl ethers (PBDEs) are receiving more and more attention. The knowledge about the distribution of PBDEs is the premise for the effective pollution control. This paper reviewed the distribution of PBDEs in the atmosphere, water, sediments, sludge, soil, plants, animals, human body and food chain all over the world. Owing to the low volatility and water solubility, the higher brominated PBDEs can be easily adsorbed to solid particles like soil, sediment and airborne particles. However, the lower brominated PBDEs are detected in all the environmental media. In living organisms, the distribution characteristics of PBDEs are depended on biological species, pollution sources, trophic levels and tissue specificity, and PBDEs are also found in human such as blood, breast milk and hair. With the prohibition of penta-, octa-, and deca-BDEs in North American and some regions of European Union, the concertrations of PBDEs in the environment have declined to some degree. However, deca-BDEs is still used in other regions around the world. Due to its persistence and long-distance transport, the control of PBDEs in the environment is still a long-term work. Thus, future research needs to focus on the level, trend, and behavior of PBDEs in the regions where they are produced and used.
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  • 收稿日期:  2017-04-19
  • 刊出日期:  2017-12-15
王森, 袁琪, 韩瑞霞, 钱亚利, 丁柳屹. 环境介质中多溴联苯醚(PBDEs)分布特征的研究进展[J]. 环境化学, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
引用本文: 王森, 袁琪, 韩瑞霞, 钱亚利, 丁柳屹. 环境介质中多溴联苯醚(PBDEs)分布特征的研究进展[J]. 环境化学, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
shu
WANG Sen, YUAN Qi, HAN Ruixia, QIAN Yali, DING Liuyi. Distribution of polybrominated diphenyl ethers (PBDEs) in the environment: A review[J]. Environmental Chemistry, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
Citation: WANG Sen, YUAN Qi, HAN Ruixia, QIAN Yali, DING Liuyi. Distribution of polybrominated diphenyl ethers (PBDEs) in the environment: A review[J]. Environmental Chemistry, 2017, 36(12): 2584-2599. doi: 10.7524/j.issn.0254-6108.2017041901
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环境介质中多溴联苯醚(PBDEs)分布特征的研究进展

  • 1.  西北大学城市与环境学院, 西安, 710127;
  • 2.  中国科学院生态环境研究中心环境化学与生态毒理学国家重点实验室, 北京, 100085
  • 收稿日期:  2017-04-19
基金项目:

国家自然科学基金（41303073），陕西省青年科技新星计划（2016KJXX-83），陕西省自然科学基础研究计划青年人才项目（2015JQ4101），陕西省教育厅科学研究项目（14JK1731）和西北大学"优秀青年学术骨干支持计划"资助.

摘要: 由多溴联苯醚（PBDEs）所引起的环境问题越来越受到社会各界的关注，了解环境介质中PBDEs的分布特征是对其污染进行有效控制的前提.本文从非生物介质（大气、水体、沉积物、污泥及土壤）和生物体内（植物、动物、人体及食物链）两方面入手，对PBDEs在世界各地不同环境介质的分布特征进行综述.高溴代PBDEs因其较低的挥发性和水溶性，极易吸附于土壤、底泥和空气悬浮颗粒等固体介质，而低溴代PBDEs在各环境介质中都有检出；生物体中PBDEs的分布特征与生物种类、污染源、营养级以及个体组织的特异性有一定关系，人体血液、母乳、头发等也检出了PBDEs.随着北美、欧盟等地区从2004年开始逐渐对五溴、八溴和十溴PBDEs实施禁用，其含量在北美和欧盟部分地区有所下降，但是由于十溴PBDEs仍在全球很多地区使用，又因其具有持久性和长距离迁移性，要实现环境介质中PBDEs含量的控制仍需要一定时间，因此未来研究仍需对PBDEs生产和使用区域开展污染水平及趋势相关研究，并对PBDEs的环境行为深入探讨.

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