碳毡和碳布2种生物阴极材料微生物燃料电池产电性能

刘松山, 陈亮, 黄满红, 郑宇. 碳毡和碳布2种生物阴极材料微生物燃料电池产电性能[J]. 环境工程学报, 2014, 8(10): 4540-4544.
引用本文: 刘松山, 陈亮, 黄满红, 郑宇. 碳毡和碳布2种生物阴极材料微生物燃料电池产电性能[J]. 环境工程学报, 2014, 8(10): 4540-4544.
Liu Songshan, Chen Liang, Huang Manhong, Zheng Yu. Electricity generation characteristics of two MFCs using carbon felt and carbon cloth as biocathode materials[J]. Chinese Journal of Environmental Engineering, 2014, 8(10): 4540-4544.
Citation: Liu Songshan, Chen Liang, Huang Manhong, Zheng Yu. Electricity generation characteristics of two MFCs using carbon felt and carbon cloth as biocathode materials[J]. Chinese Journal of Environmental Engineering, 2014, 8(10): 4540-4544.

碳毡和碳布2种生物阴极材料微生物燃料电池产电性能

  • 基金项目:

    上海市科委重点项目(09230500200)

  • 中图分类号: X382

Electricity generation characteristics of two MFCs using carbon felt and carbon cloth as biocathode materials

  • Fund Project:
  • 摘要: 为了降低构建微生物燃料电池(MFCs)的成本,比较了以碳毡和碳布作为阴极材料,在阴极利用功能微生物作为催化剂时电池的产电性能。结果表明,两电池启动时间基本相同,20 d左右达到稳定,但稳定期碳布作阴极的电池电压比碳毡作阴极的电池电压高出了60 mV左右。碳毡和碳布作阴极时,电池在10 d和20 d的最大功率密度分别由10.24和11.14 mW/m2提升到了18.18和30.15 mW/m2,相应内阻则分别由1 000和600 Ω降到了250和200Ω。循环伏安法(CV)显示两材料单独做电极时氧化还原情况相似,扫描电镜(SEM)观察到两者不同表面特性导致碳毡对污泥附着强于碳布,进而使氧气传递受到限制,产电降低。
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  • [1] 王刚,黄丽萍,张翼峰.微生物燃料电池中生物阴极的研究与应用现状.环境科学与技术,2008,31(12):101-103 Wang Gang,Huang Liping,Zhang Yifeng Study and application of biological cathode in microbial fuel cells.Environmental Science & Technology,2008,31(12):101-103(in Chinese)
    [2] Gil G.C.,Chang I.S.,Kim B.H.,et al.Operational parameters affecting the performance of a mediator-less microbial fuel cell.Biosensors and Bioelectronics,2003,18(4):327-334
    [3] 张金娜,赵庆良,尤世界,等.生物阴极微生物燃料电池不同阴极材料产电特性.高等学校化学学报,2010,31(1):162-166 Zhang Jinna,Zhao Qingliang,You Shijie,et al.Power generation in bio-cathode microbial fuel cell with different cathode materials.Chemical Journal of Chinese Universities,2010,31(1):162-166(in Chinese)
    [4] Ogah J.,Edward A.M.The use of plamwine wastewater (dregs) as substrate for the production of electric current in a microbial fuel cell.Continental J.Microbiology,2012,6(1):4-8
    [5] Bond D.R.,Holmes D.E.,Tender L.M.,et al.Electrode-reducing microorganisms that harvest energy from marine sediments.Science,2002,295(5554):483-485
    [6] Zhao F.,Harnisch F.,Schrder U.,et al.Challenges and constraints of using Oxygen cathodes in microbial fuel cells.Environmental Science & Technology,2006,40(17):5193-5199
    [7] Zhao F.,Harnisch F.,Schrder U.,et al.Application of pyrolysed iron(II) phthalocyanine and CoTMPP based oxygen reduction catalysts as cathode materials in microbial fuel cells.Electrochemistry Communications,2005,7(12):1405-1410
    [8] 陈立香,肖勇,赵峰.微生物燃料电池生物阴极.化学进展,2012,24(1):157-162 Chen Lixiang,Xiao Yong,Zhao Feng.Biocathodes in microbial fuel cells.Progress in Chemistry,2012,24(1):157-162(in Chinese)
    [9] 谢晴,王彬,杨嘉伟,等.无介体 MFC 微生物催化剂的"独立驯化"与"在线驯化"结合研究.四川大学学报(工程科学版),2011,43(1):201-207 Xie Qing,Wang Bin,Yang Jiawei,et al.Research on independent and online acclimation of bacteria catalyzer in microbial fuel cell.Journal of Sichuan University (Engineering Science Edition),2011,43(1):201-207(in Chinese)
    [10] 尹航,胡翔.不同阳极微生物燃料电池产电性能的比较.环境工程学报,2013,7(2):608-612 Yin Hang,Hu Xiang.Comparison of power generation performance of different types of anodes in microbial fuel cells.Chinese Journal of Environmental Engineering,2013,7(2):608-612(in Chinese)
    [11] 梁鹏,张玲,黄霞,等.双筒型微生物燃料电池生物阴极反硝化研究.环境科学,2010,31(8):1932-1936 Liang Peng,Zhang Ling,Huang Xia,et al.Biocathode denitrification in a two-columnar microbial fuel cell.Environmental Science,2010,31(8):1932-1936(in Chinese)
    [12] 张乐华,窦春玲,史海凤,等.在微生物燃料电池生物阴极实现硝化过程的试验研究.环境污染与防治.2012,34(9):8-12 Zhang Lehua,Dou Chunling,Shi Haifeng.Experimental study on the nitrification process in the bio-cathode of microbial fuel cells.Environmental Pollution & Control,2012,34(9):8-12(in Chinese)
    [13] Zhang F.,He Z.Integrated organic and nitrogen removal with electricity generation in a tubular dual-cathode microbial fuel cell.Process Biochemistry,2012,47(12):2146-2151
    [14] 谢珊,陈阳,梁鹏,等.好氧生物阴极型微生物燃料电池的同时硝化和产电的研究.环境科学,2010,31(7):1601-1606 Xie Shan,Chen Yang,Liang Peng,et al.Simultaneous electricity generation and nitrification in a microbial fuel cell with aerobic biocathode.Environmental Science,2010,31(7):1601-1606(in Chinese)
    [15] 倪红,熊哲,张珊,等.多孔陶粒固定化微生物效果及扫描电镜观察.湖北大学学报(自然科学版),2011,33(2):182-186 Ni Hong,Xiong Zhe,Zhang Shan,et al.Effect of porous ceramic on the immobilized microorganisms and scanning electron microscopy.Journal of Hubei University (Natural Science),2011,33(2):182-186(in Chinese)
    [16] Hernandez M.E.,Newman D.K.Extracellular electron transfer.Cellular and Molecular Life Sciences,2001,58(11):1562-1571
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出版历程
  • 收稿日期:  2013-10-17
  • 刊出日期:  2014-09-28
刘松山, 陈亮, 黄满红, 郑宇. 碳毡和碳布2种生物阴极材料微生物燃料电池产电性能[J]. 环境工程学报, 2014, 8(10): 4540-4544.
引用本文: 刘松山, 陈亮, 黄满红, 郑宇. 碳毡和碳布2种生物阴极材料微生物燃料电池产电性能[J]. 环境工程学报, 2014, 8(10): 4540-4544.
Liu Songshan, Chen Liang, Huang Manhong, Zheng Yu. Electricity generation characteristics of two MFCs using carbon felt and carbon cloth as biocathode materials[J]. Chinese Journal of Environmental Engineering, 2014, 8(10): 4540-4544.
Citation: Liu Songshan, Chen Liang, Huang Manhong, Zheng Yu. Electricity generation characteristics of two MFCs using carbon felt and carbon cloth as biocathode materials[J]. Chinese Journal of Environmental Engineering, 2014, 8(10): 4540-4544.

碳毡和碳布2种生物阴极材料微生物燃料电池产电性能

  • 1. 东华大学环境科学与工程学院, 上海 201620
基金项目:

上海市科委重点项目(09230500200)

摘要: 为了降低构建微生物燃料电池(MFCs)的成本,比较了以碳毡和碳布作为阴极材料,在阴极利用功能微生物作为催化剂时电池的产电性能。结果表明,两电池启动时间基本相同,20 d左右达到稳定,但稳定期碳布作阴极的电池电压比碳毡作阴极的电池电压高出了60 mV左右。碳毡和碳布作阴极时,电池在10 d和20 d的最大功率密度分别由10.24和11.14 mW/m2提升到了18.18和30.15 mW/m2,相应内阻则分别由1 000和600 Ω降到了250和200Ω。循环伏安法(CV)显示两材料单独做电极时氧化还原情况相似,扫描电镜(SEM)观察到两者不同表面特性导致碳毡对污泥附着强于碳布,进而使氧气传递受到限制,产电降低。

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