A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用

谢攀科, 陈东辉, 黄满红, 郑伟, 郑宇. A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用[J]. 环境工程学报, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
引用本文: 谢攀科, 陈东辉, 黄满红, 郑伟, 郑宇. A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用[J]. 环境工程学报, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
Xie Panke, Chen Donghui, Huang Manhong, Zheng Wei, Zheng Yu. Enrichment and ofloxacin degradation characteristics of nitrifying activated sludge in an A/O-MBR process[J]. Chinese Journal of Environmental Engineering, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
Citation: Xie Panke, Chen Donghui, Huang Manhong, Zheng Wei, Zheng Yu. Enrichment and ofloxacin degradation characteristics of nitrifying activated sludge in an A/O-MBR process[J]. Chinese Journal of Environmental Engineering, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314

A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用

  • 基金项目:

    国家自然科学基金资助项目(21477018,21007010)

    交通运输部科技项目(2010353343290)

  • 中图分类号: X703.1

Enrichment and ofloxacin degradation characteristics of nitrifying activated sludge in an A/O-MBR process

  • Fund Project:
  • 摘要: 采用A/O-MBR系统,逐步提高进水氨氮浓度富集了硝化活性污泥(NAS),在此基础上,考察了COD、烯丙基硫脲(ATU)、氨氮初始浓度及氨氧化速率对NAS降解氧氟沙星(OFL)的影响。结果表明:富集的NAS的氨氧化速率达到了20 mg/(g SS·h)以上,对OFL具有明显降解作用;ATU存在条件下,COD对OFL的去除作用没有影响;提高初始氨氮浓度和NAS氨氧化速率均可以提高OFL降解量;初始氨氮浓度由50 mg/提升至150 mg/L时,OFL降解量由67.26 μg/g提高到82.11 μg/g;氨氧化速率由小于2.5 mg/(g SS·h)提升至大于20 mg/(g SS·h)时,OFL降解量由30.71 μg/g提高到75.16 μg/g。
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  • [1] 王冰, 孙成, 胡冠九. 环境中抗生素残留潜在风险及其研究进展. 环境科学与技术, 2007, 30(3):108-111 Wang Bing, Sun Cheng, Hu Guanjiu. Residue antibiotics in environment:Potential risks and relevant studies. Environmental Science & Technology, 2007, 30(3):108-111(in Chinese)
    [2] Batt A. L., Kim S., Aga D. S. Enhanced biodegradation of iopromide and trimethoprim in nitrifying activated sludge. Environmental Science & Technology, 2006, 40(23):7367-7373
    [3] Verlicchi P., Aukidy M. A., Galletti A., et al. Hospital effluent:Investigation of the concentrations and distribution of pharmaceuticals and environmental risk assessment. Science of the Total Environment, 2012, 430:109-118
    [4] Verlicchi P., Galletti A., Petrovic M., et al. Hospital effluents as a source of emerging pollutants:An overview of micropollutants and sustainable treatment options. Journal of Hydology, 2010, 389(3-4):416-428
    [5] Jia Ai, Wan Yi, Xiao Yang, et al. Occurrence and fate of quinolone and fluoroquinolone antibiotics in a municipal sewage treatment plant. Water Research, 2012, 46(2):387-394
    [6] Batt A. L., Kim S., Aga D. S. Comparison of the occurrence of antibiotics in four full-scale wastewater treatment plants with varying designs and operations. Chemosphere, 2007, 68(3):428-435
    [7] Zorita S., Martensson L., Mathiasson L. Occurrence and removal of pharmaceuticals in a municipal sewage treatment system in the south of Sweden. Science of the Total Environment, 2009, 407(8):760-770
    [8] 俞慎, 王敏, 洪有为. 环境介质中的抗生素及其微生物生态效应. 生态学报, 2011, 31(15):4437-4446 Yu Shen, Wang Min, Hong Youwei. Antibiotics in environmental matrices and their effects on microbial ecosystems. Acta Ecologica Sinica, 2011, 31(15):4437-4446(in Chinese)
    [9] Kim J. Y., Ryu K., Kim E. J., et al. Degradation of bisphenol A and nonylphenol by nitrifying activated sludge. Process Biochemistry, 2007, 42(10):1470-1474
    [10] Tran N. H., Urase T., Ngo H. H., et al. Insight into metabolic and cometabolic activities of autotrophic and heterotrophic microorganisms in the biodegradation of emerging trace organic contaminants. Bioresource Technology, 2013, 146:721-731
    [11] Fernandez-Fontaina E., Omil F., Lema J. M., et al. Influence of nitrifying conditions on the biodegradation and sorption of emerging micropollutants. Water Research, 2012, 46(16):5434-5444
    [12] Dorival-García N., Zafra-Gómez A., Navalón A., et al. Removal and degradation characteristics of quinolone antibiotics in laboratory-scale activated sludge reactors under aerobic, nitrifying and anoxic conditions. Journal of Environmental Management, 2013, 120:75-83
    [13] Li Bing, Zhang Tong. Biodegradation and adsorption of antibiotics in the activated sludge process. Environmental Science & Technology, 2010, 44(9):3468-3473
    [14] Tran N. H., Urase T., Kusakabe O. The characteristics of enriched nitrifier culture in the degradation of selected pharmaceutically active compounds. Journal of Hazardous Materials, 2009, 171(1-3):1051-1057
    [15] 王彦厚, 贾雷. HPLC法测定氧氟沙星滴耳液中氧氟沙星的含量. 实用药物与临床, 2009, 12(2):107-108 Wang Yanhou, Jia Lei. Determination of ofloxacin in ofloxacin otic solution by HPLC. Practical Pharmacy and Clinical Remedies, 2009, 12(2):107-108(in Chinese)
    [16] Dorival García N., Zafra Gómez A., Navalón A., et al. Removal of quinolone antibiotics from wastewaters by sorption and biological degradation in laboratory-scale membrane bioreactors. Science of the Total Environment, 2013, 442:317-328
    [17] Shi Yijing, Wang Xinhua, Qi, Zhen, et al. Sorption and biodegradation of tetracycline by nitrifying granules and the toxicity of tetracycline on granules. Journal of Hazardous Materials, 2011, 191(1-3):103-109
    [18] Yi T., Harper Jr. W. F. The link between nitrification and biotransformation of 17α-Ethinylestradiol. Environmental Science & Technology, 2007, 41(12):4311-4316
    [19] 周玲君, 杨朝晖, 罗远玲, 等. 常温下亚硝化活性污泥的驯化及其特征. 中国给水排水, 2011, 27(7):10-14 Zhou Lingjun, Yang Zhaohui, Luo Yuanling, et al. Domestication and characteristics of short-cut nitrification activated sludge at normal temperatures. China Water & Wastewater, 2011, 27(7):10-14(in Chinese)
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  • 收稿日期:  2014-12-29
  • 刊出日期:  2016-03-18
谢攀科, 陈东辉, 黄满红, 郑伟, 郑宇. A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用[J]. 环境工程学报, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
引用本文: 谢攀科, 陈东辉, 黄满红, 郑伟, 郑宇. A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用[J]. 环境工程学报, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
Xie Panke, Chen Donghui, Huang Manhong, Zheng Wei, Zheng Yu. Enrichment and ofloxacin degradation characteristics of nitrifying activated sludge in an A/O-MBR process[J]. Chinese Journal of Environmental Engineering, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314
Citation: Xie Panke, Chen Donghui, Huang Manhong, Zheng Wei, Zheng Yu. Enrichment and ofloxacin degradation characteristics of nitrifying activated sludge in an A/O-MBR process[J]. Chinese Journal of Environmental Engineering, 2016, 10(3): 1092-1096. doi: 10.12030/j.cjee.20160314

A/O-MBR中硝化活性污泥的富集及其对氧氟沙星的降解作用

  • 1. 东华大学环境科学与工程学院,上海 201620
基金项目:

国家自然科学基金资助项目(21477018,21007010)

交通运输部科技项目(2010353343290)

摘要: 采用A/O-MBR系统,逐步提高进水氨氮浓度富集了硝化活性污泥(NAS),在此基础上,考察了COD、烯丙基硫脲(ATU)、氨氮初始浓度及氨氧化速率对NAS降解氧氟沙星(OFL)的影响。结果表明:富集的NAS的氨氧化速率达到了20 mg/(g SS·h)以上,对OFL具有明显降解作用;ATU存在条件下,COD对OFL的去除作用没有影响;提高初始氨氮浓度和NAS氨氧化速率均可以提高OFL降解量;初始氨氮浓度由50 mg/提升至150 mg/L时,OFL降解量由67.26 μg/g提高到82.11 μg/g;氨氧化速率由小于2.5 mg/(g SS·h)提升至大于20 mg/(g SS·h)时,OFL降解量由30.71 μg/g提高到75.16 μg/g。

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