青岛近岸区域典型海陆人为交互作用下酸雨的化学特征

邢建伟; 宋金明; 袁华茂; 李学刚; 李宁; 康绪明; 王启栋

doi:10.7524/j.issn.0254-6108.2017.02.2016061706

[1]

CHARLSON R, RODHE H. Factors controlling the acidity of natural rainwater[J]. Nature, 1982, 295:683-685.

[2]

CAO Y Z, WANG S Y, ZHANG G, et al. Chemical characteristics of wet precipitation at an urban site of Guangzhou, South China[J]. Atmospheric Research, 2009, 94(3):462-469.

[3]

WANG W X, WANG T. On the origin and the trend of acid precipitation in China[J]. Water, Air, and Soil Pollution, 1995, 85(4):2295-2300.

[4]

宋少杰, 陈宁, 王建华, 等. 青岛地区酸沉降现状的研究[J]. 环境科学研究, 1996, 9(5):9-12. SONG S J, CHEN N, WANG J H, et al. Study on current situation of acid deposition in Qingdao area[J]. Research of Environmental Sciences, 1996, 9(5):9-12(in Chinese).

[5]

贾洪玉, 张巧显, 邓红兵, 等. 山东省主要城市酸沉降现状及影响因素分析[J]. 环境科学, 2006, 27(12):2453-2457. JIA H Y, ZHANG Q X, DENG H B, et al. Current situation and impact factors of acid deposition in main cities of Shandong Province[J]. Environmental Science, 2006, 27(12):2453-2457(in Chinese).

[6]

王俊英, 郝欣欣, 甄文栋, 等. 青岛市降水化学组成特征及相关性分析[J]. 山东大学学报, 2006, 36(3):56-59 , 107. WANG J Y, HAO X X, ZHEN W D, et al. Characteristics and correlative analysis of chemical composition of precipitation in Qingdao City[J]. Journal of Shandong University (Engineering Science), 2006, 36(3):56-59, 107(in Chinese).

[7]

刘宝章, 李金龙, 王敬云, 等. 青岛地区边界层特征及酸雨成因[J]. 环境科学学报, 1998, 18(1):39-44. LIU B Z, LI J L, WANG J Y, et al. Character of the boundary layer and cause of acid rain in the Tsingdao area[J]. Acta Scientiae Circumstantiae, 1998, 18(1):39-44(in Chinese).

[8]

张慧明, 应金生, 林小妍, 等. 青岛市酸雨污染的状况及发展趋势[J]. 环境科学进展, 1995, 3(2):61-69. ZHANG H M, YING J S, LIN X Y, et al. The present situation and the trend of acid rain pollution in Qingdao[J]. Advances in Environmental Science, 1995, 3(2):61-69(in Chinese).

[9]

[10]

亓靓, 宋传真, 董君. 青岛市"十五"期间酸雨特征及成因浅析[J]. 环境科学与管理, 2007, 32(8):44-46. QI L, SONG C Z, DONG J. The analysis on the characteristic and causes of acid rain in Qingdao[J]. Environmental Science and Management, 2007, 32(8):44-46(in Chinese).

[11]

姜晓璐. 东、黄海的大气干、湿沉降及其对海洋初级生产力的影响[D]. 青岛:中国海洋大学, 2009:1-32. JIANG X L. Atmospheric dry and wet deposition of nutrient in East China Sea and Yellow Sea and its impact on marine primary production[D]. Qingdao:Ocean University of China, 2009:1 -32(in Chinese).

[12]

朱玉梅. 东、黄海大气沉降中营养盐的研究[D]. 青岛:中国海洋大学, 2011. ZHU Y M. Nutrients in atmospheric deposition of the Yellow and East China Sea[D]. Qingdao:Ocean University of China, 2011(in Chinese).

[13]

张占峰, 王红磊, 德力格尔, 等. 瓦里关大气降水的化学特征[J]. 大气科学学报, 2014, 37(4):502-508. ZHANG Z F, WANG H L, DELI G E, et al. Chemical characteristics of atmospheric precipitation in Waliguan[J]. Transactions of Atmospheric Sciences, 2014,37(4):502-508(in Chinese).

[14]

王艳, 葛福玲, 刘晓环, 等. 泰山降水的离子组成特征分析[J]. 中国环境科学, 2006, 26(4):422-426. WANG Y, GE F L, LIU X H, et al. Analysis of ionic composition characteristics of precipitation at Mount Taishan[J]. China Environmental Science, 2006, 26(4):422-426(in Chinese).

[15]

ZHANG X, JIANG H, ZHANG Q, et al. Chemical characteristics of rainwater in northeast China, a case study of Dalian[J]. Atmospheric Research, 2012, 116:151-160.

[16]

王志春, 丁凌云, 刘尉, 等. 广州酸雨现状及影响因素分析[J]. 热带气象学报, 2011, 27(5):717-722. WANG Z C, DING L Y, LIU W, et al. Current status and causes of acid rain in Guangzhou[J]. Journal of Tropical Meteorology, 2011, 27(5):717-722(in Chinese).

[17]

薛德强, 鹿健, 郑全岭, 等. 青岛降水的酸性分析[J]. 山东气象, 1996, 16(1) 12-14. XUE D Q, LU J, ZHENG Q L, et al. The analysis of acidity of acid rain in Qingdao[J]. Journal of Shandong Meteorology, 1996, 16(1) 12-14(in Chinese).

[18]

毕言锋. 中国东部沿海的大气营养盐干、湿沉降及其对海洋初级生产力的影响[D]. 青岛:中国海洋大学硕士学位论文, 2006:1-55. BI Y F. Atmospheric nutrient deposition at the East China coast and its impact on marine primary production[D]. Qingdao:Thesis for Master Degree of Ocean University of China, 2006:1 -55(in Chinese).

[19]

张爱群, 徐晓峰, 徐文静, 等. 北京地区酸雨概况及特征分析//中国气象学会. 中国气象学会2008年年会大气环境监测、预报与污染物控制分会场论文集[C]. 北京:中国气象学会,2008:160-163. ZHANG A Q, XU X F, XU W J, et al. The general status and characteristics of acid rain in Beijing//Chinese Meteorological Society. Proceedings of Atmospheric Environmental Monitoring, Forecast and Controlling of Pollutants of Annual Symposium for Chinese Meteorological Society, 2008[C]. Beijing:Chinese Meteorological Society, 2008 :160-163(in Chinese).

[20]

吴起鑫, 韩贵琳. 三峡水库库首地区大气降水化学特征[J]. 中国环境科学, 2012, 32(3):385-390. WU Q X, HAN G L. Chemical characteristics of rainwater collected in the head region of Three Gorges Reservoir[J]. China Environmental Science, 2012, 32(3):385-390(in Chinese).

[21]

ZHANG M Y, WANG S J, WU F C, et al. Chemical compositions of wet precipitation and anthropogenic influences at a developing urban site in southeastern China[J]. Atmospheric Research, 2007, 84(4):311-322.

[22]

刘宝章, 王敬云. 青岛地区酸雨发展时空变化研究[J]. 环境科学学报, 2000, 20(增刊):34-39. LIU B Z, WANG J Y. Study on the spatiotemporal distribution of acid rain in Qingdao region[J]. Acta Scientiae Circumstantiae, 2000 , 20(suppl):34-39(in Chinese).

[23]

TUNCER B, BAYAR B, YESILYURT C, et al. Ionic composition of precipitation at the Central Anatolia (Turkey)[J]. Atmospheric Environment, 2001, 35(34):5989-6002.

[24]

YANG F, TAN J, SHI Z B, et al. Five-year record of atmospheric precipitation chemistry in urban Beijing, China[J]. Atmospheric Chemistry and Physics, 2012, 12(4):2025-2035.

[25]

程新金, 黄美元. 降水化学特性的一种分类分析方法[J]. 气候与环境研究, 1998, 3(1):83-89. CHENG X J, HUANG M Y. A Classification method to analyze the chemical characteristics of precipitation[J]. Climatic and Environmental Research, 1998, 3(1):83-89(in Chinese).

[26]

王文兴, 许鹏举. 中国大气降水化学研究进展[J]. 化学进展, 2009, 21(2/3):266 -281. WANG W X XU P J. Research progress in precipitation chemistry in China[J]. Progress in Chemistry, 2009, 21(2/3):266-281(in Chinese).

[27]

宋金明, 詹斌秋, 李鹏程. 中国酸性沉降物致酸机理的研究//中国科协首届青年学术年会论文集(理科分册)[C]. 北京:中国科技出版社, 1992:600-610. SONG J M, ZHAN B Q, LI P C. Study of acidification mechanism for acidic deposition in China//Proceedings of the Second Academic Conference of Young Scientists of China Association for Science and Technology (Science Fascicule)[C]. Beijing:China Science and Technology Press, 1992:600 -610(in Chinese).

[28]

殷美雪. 中国中东部地区大气湿沉降中的离子化学特征[D]. 上海:上海师范大学, 2015:1-60. YIN M X. Chemical characteristics of ions in atmospheric wet deposition in the mid-eastern China[D]. Shanghai:Shanghai Normal University, 2015:1 -60(in Chinese).

[29]

FENG Z W, HUANG Y Z, FENG Y W, et al. Chemical composition of precipitation in Beijing area, Northern China[J]. Water, Air, and Soil Pollution, 2001, 125(1):345-356.

[30]

TANG A H, ZHUANG G S, WANG Y, et al. The chemistry of precipitation and its relation to aerosol in Beijing[J]. Atmospheric Environment, 2005, 39(19):3397-3406.

[31]

BAI L, WANG Z L. Anthropogenic influence on rainwater in the Xi'an City, Northwest China:Constraints from sulfur isotope and trace elements analyses[J]. Journal of Geochemical Exploration, 2014, 137:65-72.

[32]

XIAO J. Chemical composition and source identification of rainwater constituents at an urban site in Xi'an[J]. Environmental Earth Sciences, 2016, 75(3):1-12.

[33]

WANG Y S, YU W P, PAN Y P, et al. Acid neutralization of precipitation in Northern China[J]. Journal of the Air & Waste Management Association, 2012, 62(2):204-211.

[34]

王文兴, 丁国安. 中国降水酸度和离子浓度的时空分布[J]. 环境科学研究, 1997, 10(2):1-7. WANG W X, DING G A. The geographical distribution of ion concentration in precipitation over China[J]. Research of Environmental Sciences, 1997, 10(2):1-7(in Chinese).

[35]

张新民, 柴发合, 王淑兰, 等. 中国酸雨研究现状[J]. 环境科学研究, 2010, 23(5):527-532. ZHANG X M, CHAI F H, WANG S L, et al. Research progress of acid precipitation in China[J]. Research of Environmental Sciences, 2010, 23(5):527-532(in Chinese).

[36]

[37]

[38]

魏巍. 青岛市酸雨影响因素分析及降水酸度预测[D]. 青岛:中国海洋大学, 2008:1-70. WEI W. The influencing factors analysis of acid rain and forecast of precipitation acidity in Qingdao[D]. Qingdao:Ocean University of China, 2008:1 -70(in Chinese).

[39]

宋金明, 李鹏程, 詹斌秋. 大气污染物质SO₂对雾水酸度的控制作用[J]. 海洋科学, 1994, 18(5):44-49. SONG J M, LI P C, ZHAN B Q. Controlling effect of atmospheric pollutant SO₂ on fogwater acidity[J]. Marine Sciences, 1994, 18(5):44-49(in Chinese).

[40]

刘宝章, 李金龙, 王敬云, 等. 青岛酸雨天气边界层气象特征[J]. 中国环境科学, 1997,17(2):103-107. LIU B Z, LI J L, WANG J Y, et al. Meteorological features of the boundary layer for the weather of acid rain in Qingdao[J]. China Environmental Science, 1997,17(2):103-107(in Chinese).

[41]

王文兴. 中国酸雨成因研究[J]. 中国环境科学, 1994, 14(5):323-328. WANG W X. Study on the origin of acid rain formation in China[J]. China Environmental Science, 1994, 14(5):323-328(in Chinese).

[42]

朱彤. 城市与区域大气复合污染//戴树桂. 环境化学进展[M]. 北京:化学工业出版社, 2005:1-17. ZHU T. Combined air pollution in city and region//. DAI S G. Advances in Environmental Chemistry[M]. Beijing:Chemical Industry Press, 2005:1 -17(in Chinese).

[43]

马奇菊, 胡敏, 田旭东, 等. 青岛近岸海域二甲基硫排放和大气中二甲基硫浓度变化[J]. 环境科学, 2004, 25(1):20-24. MA Q J, HU M, TIAN X D, et al. Dimethylsulfide emission in Qingdao near-shore waters and atmospheric dimethylsulfide concentration variation[J]. Environmental Science, 2004,25(1):20-24(in Chinese).

[44]

田旭东, 胡敏, 马奇菊. 青岛环境大气和海洋表层水中挥发性硫化物的测定[J]. 环境科学学报, 2005, 25(1):30-33. TIAN X D, HU M, MA Q J. Determination of volatile sulfur compounds in the atmosphere and surface seawater in Qingdao[J]. Acta Scientiae Circumstantiae, 2005, 25(1):30-33(in Chinese).

[45]

胡敏, 唐孝炎, 李金龙, 等. 胶州湾海水中二甲基硫的测定[J]. 环境科学学报, 1997, 17(1):110-115. HU M, TANG X Y, LI J L, et al. Dimethylsulfide in sea water in the Gulf of Jiaozhou[J]. Acta Scientiae Circumstantiae, 1997, 17(1):110-115(in Chinese).

[46]

LU X W, LI L Y, LI N, et al. Chemical characteristics of spring rainwater of Xi'an city, NW China[J]. Atmospheric Environment, 2011, 45(28):5058-5063.

[47]

CAO J J, TIE X X, DABBERDT W F, et al. On the potential high acid deposition in northeastern China[J]. Journal of Geophysical Research:Atmospheres, 2013, 118(10):4834-4846.

[48]

XU Z F, WU Y, LIU W J, et al. Chemical composition of rainwater and the acid neutralizing effect at Beijing and Chizhou city, China[J]. Atmospheric Research, 2015, 164:278-285.

[49]

WU D, WANG S G, XIA J R, et al. The influence of dust events on precipitation acidity in China[J]. Atmospheric Environment, 2013, 79:138-146.

[50]

刘素美, 黄薇文, 张经, 等. 青岛地区大气沉降物中化学成分研究2.常量组分[J]. 海洋环境科学, 1993, 12(3/4):89 -98. LIU S M, HUANG W W ZHANG J, et al. Study on the chemical components of atmospheric deposition matters in Qingdao 2. Bulk component[J]. Marine Environmental Science, 1993, 12(3/4):89-98(in Chinese).

[51]

AL-KHASHMAN O A. Chemical characteristics of rainwater collected at a western site of Jordan[J]. Atmospheric Research, 2009, 91(1):53-61.

[52]

KEENE W C, PSZENNY A A P, GALLOWAY J N, et al. Sea-salt corrections and interpretation of constituent ratios in marine precipitation[J]. Journal of Geophysical Research:Atmospheres, 1986, 91(D6):6647-6658.

[53]

TAYLOR S. Abundance of chemical elements in the continental crust:a new table[J]. Geochimica et Cosmochimica Acta, 1964, 28(8):1273-1285.

[54]

LI Y C, ZHANG M, SHU M, et al. Chemical characteristics of rainwater in Sichuan basin, a case study of Ya'an[J]. Environmental Science and Pollution Research, 2016:23(13):13088-13099.

[55]

DAS R, DAS S N, MISRA V N. Chemical composition of rainwater and dustfall at Bhubaneswar in the east coast of India[J]. Atmospheric Environment, 2005, 39(32):5908-5916.

[56]

肖辉, 沈志来, 黄美元. 西太平洋热带海域降水化学特征[J]. 环境科学学报, 1993, 13(2):143-149. XIAO H, SHEN Z L, HUANG M Y. Chemical characteristics of tropical western Pacific precipitation[J]. Acta Scientiae Circumstantiae, 1993, 13(2):143-149(in Chinese).

[57]

张金良, 于志刚, 张经, 等. 黄海西部大气湿沉降(降水)的pH与主要酸碱离子的关系[J]. 海洋环境科学, 2000, 19(3):30-34. ZHANG J L, YU Z G, ZHANG J, et al. Relation of pH and major acid and alkaline ions in atmospheric wet deposition (precipitation) of Western Yellow Sea[J]. Marine Environmental Science, 2000, 19(3):30-34(in Chinese).

[58]

武瑶, 徐志方. 大气降水中稳定同位素研究进展[J]. 地球与环境, 2013, 41(6):688-695. WU Y, XU Z F. Progress in research on stable isotopes in precipitation in China:A review[J]. Earth and Environment, 2013, 41(6):688-695(in Chinese).

[59]

XIAO H W, XIE L H, LONG A M, et al. Use of isotopic compositions of nitrate in TSP to identify sources and chemistry in South China Sea[J]. Atmospheric Environment, 2015, 109:70-78.

[60]

李亲凯, 杨周, 黄俊, 等. 大气颗粒物稳定同位素组成的研究进展[J]. 生态学杂志, 2016, 35(4):1063-1071. LI Q K, YANG Z, HUANG J, et al. A review of stable isotopic compositions of atmospheric particulate matter[J]. Chinese Journal of Ecology, 2016, 35(4):1063-1071(in Chinese).

[61]

李佩霖, 傅平青, 康世昌, 等. 大气气溶胶中的氮:化学形态与同位素特征研究进展[J]. 环境化学, 2016, 35(1):1-10. LI P L, FU P Q, KANG S C, et al. Research progress on nitrogen in atmospheric aerosol:Chemical speciation and isotopic characteristics[J]. Environmental Chemistry, 2016, 35(1):1-10(in Chinese).

[62]

宋宇然. 青岛地区大气湿沉降的研究[D]. 青岛:中国海洋大学, 2006:1-59. SONG Y R. The study on atmospheric wet deposition in Qingdao[D]. Qingdao:Thesis for Master Degree of Ocean University of China, 2006:1 -59(in Chinese).

[63]

XU H, BI X H, FENG Y C, et al. Chemical composition of precipitation and its sources in Hangzhou, China[J]. Environmental Monitoring and Assessment, 2011, 183(1/4):581-592.

[64]

WANG H, HAN G L. Chemical composition of rainwater and anthropogenic influences in Chengdu, Southwest China[J]. Atmospheric Research, 2011, 99(2):190-196.

[65]

HUANG K, ZHUANG G S, XU C, et al. The chemistry of the severe acidic precipitation in Shanghai, China[J]. Atmospheric Research, 2008, 89(1):149-160.

[66]

宋金明, 李鹏程, 詹斌秋. 青岛雾水中的氯离子[J]. 海洋环境科学, 1992, 11(4):14-22. SONG J M, LI P C, ZHAN B Q. The chloridion in fog of Qingdao[J]. Marine Environmental Science, 1992, 11(4):14-22(in Chinese).

[67]

宋金明. 海洋环境中硫的存在形式[J]. 环境化学, 1990, 9(6):59-64. SONG J M. Species of sulfur in marine environments[J]. Environmental Chemistry, 1990, 9(6):59-64(in Chinese).

[68]

AVERY G B, KIEBER R J, WITT M, et al. Rainwater monocarboxylic and dicarboxylic acid concentrations in southeastern North Carolina, USA, as a function of air-mass back-trajectory[J]. Atmospheric Environment, 2006, 40(9):1683-1693.

[69]

徐刚, 李心清, 吕迎春, 等. 大气降水中低分子有机酸的季节变化及对酸雨形成的贡献(以贵阳市和尚重镇为例)[J]. 科学通报, 2009, 54(17):2568-2573. XU G, LI X Q, LV Y C, et al. Seasonal variations of carboxylic acids and their contributions to the rainwater acidity:A case study of Guiyang City and Shangzhong Town, China[J]. Chinese Science Bulletin, 2009, 54(17):2568-2573(in Chinese).

[70]

ZHANG Y L, LEE X Q, CAO F, et al. Seasonal variation and sources of low molecular weight organic acids in precipitation in the rural area of Anshun[J]. Chinese Science Bulletin, 2011, 56(10):1005-1010.

[71]

GALLOWAY J N, LIKENS G E, KEENE W C, et al. The composition of precipitation in remote areas of the world[J]. Journal of Geophysical Research:Oceans, 1982, 87(C11):8771-8786.