朔州市夏季环境空气中VOCs的污染特征及来源解析

李如梅; 武媛媛; 彭林; 马青兰; 李颖慧; 王海京; 牟玲; 闫雨龙; 白慧玲

doi:10.7524/j.issn.0254-6108.2017.05.2016111603

[1]

VARUTBANGKUL V, BRECHTEL F J, BAHREINI R, et al. Hygroscopicity of secondary organic aerosols formed by oxidation of cycloalkenes, monoterpenes, sesquiterpenes, and related compounds[J]. Atmospheric Chemistry & Physics, 1977, 32(6): 466-467.

[2]

HATFIELD M L, HARTZ K E H. Secondary organic aerosol from biogenic volatile organic compound mixtures[J]. Atmospheric Environment, 2011, 45(13): 2211-2219.

[3]

罗达通,高健,王淑兰,等. 北京秋季大气挥发性有机物及相关污染物特征分析[J]. 中国科学院大学学报, 2014, 31(3): 329-336. LUO D T, GAO J, WANG S L, et al. Characteristics of volatile organic compounds and relative pollutants observed in autumn in Beijing[J].Journal of University of Chinese Academy of Sciences,2014, 31(3): 329-336(in Chinese).

[4]

张俊刚,王跃思,王珊,等. 京津地区大气中非甲烷烃(NMHCs)质量浓度水平和反应活性研究[J]. 环境科学研究, 2008, 21(5): 158-162. ZHANG J G, WANG Y S, WANG S, et al. Ambient mass concentration and reactivity of non-methane hydrocarbons (NMHCs) in Beijing and Tianjin cities[J].Research of Environmental Sciences,2008, 21(5): 158-162(in Chinese).

[5]

卢学强,韩萌,冉靓,等. 天津中心城区夏季非甲烷有机化合物组成特征及其臭氧产生潜力分析[J]. 环境科学学报, 2011, 31(2): 373-380. LU X Q, HAN M, RAN J, et al. Characteristics of nonmethane organic compounds and their ozone formation potentials in downtown Tianjin in summer[J].Acta Scientiae Circumstantiae,2011, 31(2): 373-380(in Chinese).

[6]

WANG M, SHAO M, LU S H, et al. Evidence of coal combustion contribution to ambient VOCs during winter in Beijing[J]. Chinese Chemical Letters, 2013, 24 (9): 829-832.

[7]

郑伟巍,毕晓辉,吴建会,等. 宁波市大气挥发性有机物污染特征及关键活性组分[J]. 环境科学研究, 2014,27 (12): 1411-1419. ZHENG W W, BI X H, WU J H, et al. Pollution characteristics and key reactive species of ambient VOCs in Ningbo City[J]. Research of Environmental Sciences, 2014, 27(12): 1411-1419(in Chinese).

[8]

杨辉,朱彬,高晋徽,等. 南京市北郊夏季挥发性有机物的源解析[J]. 环境科学, 2013, 34(12): 4519-4528. YANG H, ZHU B, GAO J H, et al. Source apportionment of VOCs in the northern suburb of Nanjing in Summer[J]. Environmental Science,2013, 34(12): 4519-4528(in Chinese).

[9]

CAI C, GENG F, TIE X, et al. Characteristics and source apportionment of VOCs measured in Shanghai, China[J]. Atmospheric Environment, 2010, 44(38): 5005-5014.

[10]

苏雷燕. 上海市城区大气VOCs的变化特征及反应活性的初步研究[D]. 上海: 华东理工大学, 2012. SU L Y. A preliminary study of ambient VOCs variation and chemical reactivity in the urban area of Shanghai,China[D]. Shanghai: East China University of Science and Technology,2012(in Chinese).

[11]

杨笑笑,汤莉莉,张运江,等. 南京夏季市区 VOCs 特征及 O₃生成潜势的相关性分析[J]. 环境科学, 2016, 37(2): 443-451. YANG X X, TANG L L, ZHANG Y J, et al. Correlation analysis between characteristics of VOCs and ozone formation potential in Summer in Nanjing Urban District[J]. Environmental Science,2016, 37(2): 443-451(in Chinese).

[12]

朱少峰,黄晓锋,何凌燕,等. 深圳大气VOCs浓度的变化特征与化学反应活性[J]. 中国环境科学, 2012, 32(12): 2140-2148. ZHU S F, HUANG X F, HE L Y, et al. Variation characteristics and chemical reactivity of ambient VOCs in Shenzhen[J]. China Environmental Science,2012, 32(12): 2140-2148(in Chinese).

[13]

解鑫,邵敏,刘莹,等. 大气挥发性有机物的日变化特征及在臭氧生成中的作用——以广州夏季为例[J]. 环境科学学报, 2009, 29(1): 54-62. XIE X, SHAO M, LIU Y, et al. The diurnal variation of ambient VOCs and their role in ozone formation:Case study in summer in Guangzhou[J]. Acta Scientiae Circumstantiae,2009, 29(1): 54-62(in Chinese).

[14]

邓雪娇,周秀骥,吴兑,等. 珠江三角洲大气气溶胶对地面臭氧变化的影响[J]. 中国科学:地球科学, 2011, 41(1): 93-102. DENG X J, ZHOU X J, WU D, et al. Effect of atmospheric aerosol on surface ozone variation over the Pearl River Delta region[J].Science China Earth Sciences,2011, 41(1): 93-102(in Chinese).

[15]

李雷,李红,王学中,等. 广州市中心城区环境空气中挥发性有机物的污染特征与健康风险评价[J]. 环境科学, 2013, 34(12): 4558-4564. LI L, LI H, WANG X Z, et al. Pollution characteristics and health risk assessment of atmospheric vocs in the downtown area of Guangzhou,China[J]. ENVIRONMENTAL SCIENCE,2013, 34(12): 4558-4564(in Chinese).

[16]

李丽娟. 朔州市城区大气挥发性有机物的特征研究及来源分析[D]. 太原: 太原理工大学, 2015. LI L J. A Prelimary study on characteristic and source of volatile organic compounds in the urban area of Shuozhou[D]. Taiyuan: Taiyuan University of Technology,2015(in Chinese).

[17]

乔月珍,王红丽,黄成,等. 机动车尾气排放VOCs源成分谱及其大气反应活性[J]. 环境科学, 2012, 33(4): 1071-1079. QIAO Y Z, WANG H L, HUANG C, et al. Source profile and chemical reactivity of volatile organic compounds from vehicle exhaust[J]. Environmental Science,2012, 33(4): 1071-1079(in Chinese).

[18]

王倩,王红丽,周来东,等. 成都市夏季大气挥发性有机物污染及其对二次有机气溶胶生成的贡献[J]. 环境污染与防治, 2015, 37(7): 6-12. WANG Q, WANG H L, ZHOU L D, et al. Pollution of volatile organic compounds and their contribution to the secondary organic aerosol formation in summer of Chendu[J].Environmental Pollution & Control,2015, 37(7): 6-12(in Chinese).

[19]

董海燕,朱玲,边玮瓅,等. 天津市滨海新区夏季挥发性有机物的污染特征分析[J]. 环境污染与防治, 2016, 38(5): 77-81. DONG H Y, ZHU L, BIAN W L, et al. Pollution characteristics of volatile organic compounds in the summer of Binhai New Aera,Tianjin[J]. Environmental Pollution & Control,2016, 38(5): 77-81(in Chinese).

[20]

温彦平,闫雨龙,李丽娟,等. 太原市夏季挥发性有机物污染特征及来源分析[J]. 太原理工大学学报, 2016, 47(3): 331-336. WEN Y P, YAN Y L, LI L J, et al. Pollution characteristics and source analysis of volatile organic compounds in Summer in Taiyuan[J].JOURNAL OF TAIYUAN UNIVERSITY OF TECHNOLOGY,2016, 47(3): 331-336(in Chiese).

[21]

刘泽常,张帆,侯鲁健,等. 济南市夏季环境空气VOCs污染特征研究[J]. 环境科学, 2012, 33(10): 3656-3661. LIU Z C, ZHANG F, HOU L J, et al. Pollution characteristics of VOCs in Ambient Air of Ji'nan City in Summer[J]. Environmental Science,2012, 33(10): 3656-3661(in Chinese).

[22]

ATKINSON R. Atmospheric chemistry of VOCs and NO_<i>x[J]. Atmospheric Environment. 2000, 34(12-14):2063-2101.

[23]

TANG J H, CHAN L Y, CHAN C Y, et al. Characteristics and diurnal variations of NMHCs at urban, suburban, and rural sites in the Pearl River Delta and a remote site in South China[J]. Atmospheric Environment. 2007, 41(38): 8620-8632.

[24]

LIU Y, SHAO M, FU L, et al. Source profiles of volatile organic compounds (VOCs) measured in China: Part I[J]. Atmospheric Environment. 2008, 42(25): 6247-6260.

[25]

JOBSON B T, PARRISH D D, GOLDAN P, et al. Spatial and temporal variability of nonmethane hydrocarbon mixing ratios and their relation to photochemical lifetime[J]. Journal of Geophysical Research. 1995, 32(1031): 13557-13568.

[26]

CHANG C, WANG J, LIU S, et al. Assessment of vehicular and non-vehicular contributions to hydrocarbons using exclusive vehicular indicators[J]. Atmospheric Environment. 2006, 40(33): 6349-6361.

[27]

THURSTON G D, SPENGLER J D. A quantitative assessment of source contributions to inhalable particulate matter pollution in metropolitan Boston[J]. Atmospheric Environment. 1985, 19(1): 9-25.

[28]

莫梓伟,邵敏,陆思华. 中国挥发性有机物(VOCs)排放源成分谱研究进展[J]. 环境科学学报, 2014, 34(9): 2179-2189. MO Z W, SHAO M, LU S H. Review on volatile organic compounds (VOCs) source profiles measured in China[J].Acta Scientiae Circumstantiae,2014, 34(9): 2179-2189(in Chinese).

[29]

谢扬飏,邵敏,陆思华,等. 北京市园林绿地植被挥发性有机物排放的估算[J]. 中国环境科学, 2007, 27(4): 498-502. XIE Y Y, SHAO M, LU S H, et al. The estimation of volatile organic compounds emission from landscape plants in Beijing[J]. China Environmental Science,2007, 27(4):498-502(in Chinese).

[30]

DRAXLER R R, HESS G D, DRAXLER R R. An overview of the HYSPLIT_4 modelling system for trajectories[J]. Australian Meteorological Magazine, 1998, 47(4): 295-308.

[31]

YU S, MATHUR R, KANG D, et al. A study of the ozone formation by ensemble back trajectory-process analysis using the Eta-CMAQ forecast model over the northeastern U.S. during the 2004 ICARTT period[J]. Atmospheric Environment, 2009, 43(2): 355-363.

[32]

CARTER W P L. Development of ozone reactivity scales for volatile organic compounds[J]. Air Repair, 1994, 44(7): 881-899.

[33]

GROSJEAN D. In situ organic aerosol formation during a smog episode: Estimated production and chemical functionality[J]. Atmospheric Environment, 1992, 26(6): 953-963.

[34]

GROSJEAN D, SEINFELD J H. Parameterization of the formation potential of secondary organic aerosols[J]. Atmospheric Environment, 1989, 23(8): 1733-1747.