我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度

余龙飞, 李炳文, 张逸, 王章玮. 我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度[J]. 环境化学, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
引用本文: 余龙飞, 李炳文, 张逸, 王章玮. 我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度[J]. 环境化学, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
YU Longfei, LI Bingwen, ZHANG Yi, WANG Zhangwei. Natural abundance of nitrogen isotopes for ammonium nitrogen in rainfall and throughfall at some sites in China[J]. Environmental Chemistry, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
Citation: YU Longfei, LI Bingwen, ZHANG Yi, WANG Zhangwei. Natural abundance of nitrogen isotopes for ammonium nitrogen in rainfall and throughfall at some sites in China[J]. Environmental Chemistry, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001

我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度

  • 基金项目:

    中国科学院知识创新方向性项目(K2CX2-YW-GJ01)

    中国科学院国际合作项目(GJHZ1205)

    国家重大基础研究(973计划)项目(2005CB422206)资助.

Natural abundance of nitrogen isotopes for ammonium nitrogen in rainfall and throughfall at some sites in China

  • Fund Project:
  • 摘要: 在我国7个站点采集了降雨和森林穿冠水样品,分析了铵态氮的同位素丰度.结果表明,各站点降雨中铵态氮δ15N的平均值为-8.67‰至-3.66‰,其中杭州近郊梅家坞降水样品中铵态氮δ15N平均值最低,贵州雷公山降雨样品中铵态氮δ15N平均值最高.城市穿冠水中铵态氮δ15N值要明显高于降雨,而郊区和背景地区穿冠水中铵态氮δ15N值略高于降雨,这可能是由于城市地区林冠层富集有更多的大气颗粒物并通过冲刷过程进入穿冠水所致,因为大气颗粒物中铵态氮通常富集N.
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  • [1] Ding W, Cai Y, Cai Z, et al. Nitrous oxide emissions from an intensively cultivated maize-wheat rotation soil in the North China Plain[J]. Science of the Total Environment, 2007, 373: 501-511
    [2] Zhang Y, Liu J, Mu Y, et al. Emissions of nitrous oxide, nitrogen oxides and ammonia from a maize field in the North China Plain[J]. Atmospheric Environment, 2011, 45: 2956-2661
    [3] Galloway J, Dentenber F, Capone D, et al. Nitrogen cycles: Past, present, and future[J]. Biogeochemistry, 2004, 70: 153-226
    [4] 周薇,王兵,李钢铁. 大气氮沉降对森林生态系统影响的研究进展[J]. 中央名族大学学报,2010,19(1):34-40
    [5] Zhang Y, Dore A, Ma L, et al. Agricultural ammonia emissions inventory and spatial distribution in the North China Plain[J]. Environmental Pollution, 2010, 158: 490-501
    [6] 罗绪强,王世杰,刘秀明. 稳定氮同位素在环境污染示踪中的应用进展[J]. 矿物岩石地球化学通报,2007,26(3):295-299
    [7] Freyer H. Seasonal trends of NH4 and NO3 nitrogen isotope composition in rain collected at Jülich, Germany[J]. Tellus, 1978, 30: 83-92
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    [9] Garten J Jr. Nitrogen isotope composition of ammonium and nitrate in bulk precipitation and forest throughfall[J]. International Journal of Analytical Chemistry, 1992, 47: 33-45
    [10] 曾明,余龙飞,张逸,等. 天然水体中铵态和硝态氮δ15N的测定[J]. 环境化学,2013,32(8):1486-1490
    [11] Silva S, Kendall C, Wilkison D, et al. A new method for collection of nitrate from fresh water and the analysis of nitrogenand oxygen isotope ratios[J]. Journal of Hydrology, 2000, 228 (1/2): 22-36
    [12] 蒲维维,张小玲,徐敬,等. 北京地区酸雨特征及影响因素[J]. 应用气象学报,2010,21:464-471
    [13] 彭应登,杨明珍,申立贤. 北京氨源排放及其对二次粒子生成的影响[J]. 环境科学,2000,21(1):101-103
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  • 收稿日期:  2012-05-25
余龙飞, 李炳文, 张逸, 王章玮. 我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度[J]. 环境化学, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
引用本文: 余龙飞, 李炳文, 张逸, 王章玮. 我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度[J]. 环境化学, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
YU Longfei, LI Bingwen, ZHANG Yi, WANG Zhangwei. Natural abundance of nitrogen isotopes for ammonium nitrogen in rainfall and throughfall at some sites in China[J]. Environmental Chemistry, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001
Citation: YU Longfei, LI Bingwen, ZHANG Yi, WANG Zhangwei. Natural abundance of nitrogen isotopes for ammonium nitrogen in rainfall and throughfall at some sites in China[J]. Environmental Chemistry, 2013, 32(9): 1599-1603. doi: 10.7524/j.issn.0254-6108.2013.09.001

我国一些站点降雨和森林穿冠水中铵态氮的同位素丰度

  • 1. 中国科学院生态环境研究中心, 北京, 100085
基金项目:

中国科学院知识创新方向性项目(K2CX2-YW-GJ01)

中国科学院国际合作项目(GJHZ1205)

国家重大基础研究(973计划)项目(2005CB422206)资助.

摘要: 在我国7个站点采集了降雨和森林穿冠水样品,分析了铵态氮的同位素丰度.结果表明,各站点降雨中铵态氮δ15N的平均值为-8.67‰至-3.66‰,其中杭州近郊梅家坞降水样品中铵态氮δ15N平均值最低,贵州雷公山降雨样品中铵态氮δ15N平均值最高.城市穿冠水中铵态氮δ15N值要明显高于降雨,而郊区和背景地区穿冠水中铵态氮δ15N值略高于降雨,这可能是由于城市地区林冠层富集有更多的大气颗粒物并通过冲刷过程进入穿冠水所致,因为大气颗粒物中铵态氮通常富集N.

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