宝鸡市秋季清洁和污染时段水溶性离子污染特征及来源解析

周变红; 冯瞧; 王锦; 李春燕; 许东东; 李建军

doi:10.7524/j.issn.0254-6108.2021102901

[1]

王跃思, 张军科, 王莉莉, 等. 京津冀区域大气霾污染研究意义、现状及展望 [J]. 地球科学进展, 2014, 29(3): 388-396. doi: 10.11867/j.issn.1001-8166.2014.03.0388 WANG Y S, ZHANG J K, WANG L L, et al. Researching significance, status and expectation of haze in Beijing-Tianjin-Hebei region [J]. Advances in Earth Science, 2014, 29(3): 388-396(in Chinese). doi: 10.11867/j.issn.1001-8166.2014.03.0388

[2]

ZHENG G J, DUAN F K, SU H, et al. Exploring the severe winter haze in Beijing: The impact of synoptic weather, regional transport and heterogeneous reactions [J]. Atmospheric Chemistry and Physics, 2015, 15(6): 2969-2983. doi: 10.5194/acp-15-2969-2015

[3]

MAJI K J, YE W F, ARORA M, et al. PM_2.5 related health and economic loss assessment for 338 Chinese cities[J]. Environment International, 2018, 121(Pt 1): 392-403.

[4]

LIU F, TAN Q W, JIANG X, et al. Effects of relative humidity and PM_2.5 chemical compositions on visibility impairment in Chengdu, China [J]. Journal of Environmental Sciences, 2019, 86: 15-23. doi: 10.1016/j.jes.2019.05.004

[5]

HUANG F, ZHOU J B, CHEN N, et al. Chemical characteristics and source apportionment of PM_2.5 in Wuhan, China [J]. Journal of Atmospheric Chemistry, 2019, 76(3): 245-262. doi: 10.1007/s10874-019-09395-0

[6]

LI X R, WANG Y S, GUO X Q, et al. Seasonal variation and source apportionment of organic and inorganic compounds in PM_2.5 and PM₁₀ particulates in Beijing, China [J]. Journal of Environmental Sciences, 2013, 25(4): 741-750. doi: 10.1016/S1001-0742(12)60121-1

[7]

LIU X Y, WANG M S, PAN X L, et al. Chemical formation and source apportionment of PM_2.5 at an urban site at the southern foot of the Taihang mountains [J]. Journal of Environmental Sciences, 2021, 103: 20-32. doi: 10.1016/j.jes.2020.10.004

[8]

王德羿, 王体健, 韩军彩, 等. “2+26”城市大气重污染下PM_2.5来源解析 [J]. 中国环境科学, 2020, 40(1): 92-99. doi: 10.3969/j.issn.1000-6923.2020.01.010 WANG D Y, WANG T J, HAN J C, et al. Source apportionment of PM_2.5 under heavy air pollution conditions in “2+26” cities [J]. China Environmental Science, 2020, 40(1): 92-99(in Chinese). doi: 10.3969/j.issn.1000-6923.2020.01.010

[9]

SHEN Z X, SUN J, CAO J J, et al. Chemical profiles of urban fugitive dust PM_2.5 samples in Northern Chinese cities [J]. Science of the Total Environment, 2016, 569/570: 619-626. doi: 10.1016/j.scitotenv.2016.06.156

[10]

周变红, 王锦, 曹夏, 等. 宝鸡市冬季PM_2.5中元素污染特征及健康风险评估 [J]. 生态毒理学报, 2020, 15(4): 299-311. ZHOU B H, WANG J, CAO X, et al. Characteristics and health risk assessments of elements in PM_2.5 during winter in Baoji city [J]. Asian Journal of Ecotoxicology, 2020, 15(4): 299-311(in Chinese).

[11]

曹夏, 周变红, 王锦, 等. 西安城区黑碳气溶胶的污染特征及来源解析 [J]. 环境化学, 2020, 39(11): 3072-3082. doi: 10.7524/j.issn.0254-6108.2020061501 CAO X, ZHOU B H, WANG J, et al. Characteristics and source analysis of black carbon aerosol in Xi'an Urban Area [J]. Environmental Chemistry, 2020, 39(11): 3072-3082(in Chinese). doi: 10.7524/j.issn.0254-6108.2020061501

[12]

HAN X K, GUO Q J, LIU C Q, et al. Effect of the pollution control measures on PM_2.5 during the 2015 China Victory Day Parade: Implication from water-soluble ions and sulfur isotope [J]. Environmental Pollution, 2016, 218: 230-241. doi: 10.1016/j.envpol.2016.06.038

[13]

LIU P F, ZHANG C L, MU Y J, et al. The possible contribution of the periodic emissions from farmers' activities in the North China Plain to atmospheric water-soluble ions in Beijing [J]. Atmospheric Chemistry and Physics, 2016, 16(15): 10097-10109. doi: 10.5194/acp-16-10097-2016

[14]

TIAN M, LIU Y, YANG F M, et al. Increasing importance of nitrate formation for heavy aerosol pollution in two megacities in Sichuan Basin, southwest China [J]. Environmental Pollution, 2019, 250: 898-905. doi: 10.1016/j.envpol.2019.04.098

[15]

张棕巍, 胡恭任, 于瑞莲, 等. 厦门市大气PM_2.5中水溶性离子污染特征及来源解析 [J]. 中国环境科学, 2016, 36(7): 1947-1954. doi: 10.3969/j.issn.1000-6923.2016.07.004 ZHANG Z W, HU G R, YU R L, et al. Characteristics and sources apportionment of water-soluble ions in PM_2.5 of Xiamen City, China [J]. China Environmental Science, 2016, 36(7): 1947-1954(in Chinese). doi: 10.3969/j.issn.1000-6923.2016.07.004

[16]

郑敬茹, 瞿厚淑, 付山, 等. 黄石市大气PM_2.5中水溶性离子浓度特征及来源分析 [J]. 环境科学研究, 2019, 32(7): 1170-1178. ZHENG J R, QU H S, FU S, et al. Characteristics and source analysis of water-soluble inorganic ions in PM_2.5 in Huangshi city [J]. Research of Environmental Sciences, 2019, 32(7): 1170-1178(in Chinese).

[17]

王念飞, 陈阳, 郝庆菊, 等. 苏州市PM_2.5中水溶性离子的季节变化及来源分析 [J]. 环境科学, 2016, 37(12): 4482-4489. WANG N F, CHEN Y, HAO Q J, et al. Seasonal variation and source analysis of the water-soluble inorganic ions in fine particulate matter in Suzhou [J]. Environmental Science, 2016, 37(12): 4482-4489(in Chinese).

[18]

ZHOU J B, XING Z Y, DENG J J, et al. Characterizing and sourcing ambient PM_2.5 over key emission regions in China Ⅰ: Water-soluble ions and carbonaceous fractions [J]. Atmospheric Environment, 2016, 135: 20-30. doi: 10.1016/j.atmosenv.2016.03.054

[19]

WU C, WANG G H, WANG J Y, et al. Chemical characteristics of haze particles in Xi'an during Chinese Spring Festival: Impact of fireworks burning [J]. Journal of Environmental Sciences, 2018, 71: 179-187. doi: 10.1016/j.jes.2018.04.008

[20]

黄含含, 王羽琴, 李升苹, 等. 西安市PM_2.5中水溶性离子的季节变化特征 [J]. 环境科学, 2020, 41(6): 2528-2535. HUANG H H, WANG Y Q, LI S P, et al. Seasonal variation of water-soluble ions in PM_2.5 in Xi'an [J]. Environmental Science, 2020, 41(6): 2528-2535(in Chinese).

[21]

ZHANG T. , CAO J J, TIE X X, et al. Water-soluble ions in atmospheric aerosols measured in Xi'an, China: Seasonal variations and sources [J]. Atmospheric Research, 2011, 102(1-2): 110-119. doi: 10.1016/j.atmosres.2011.06.014

[22]

NENES A, PANDIS S N, PILINIS C. ISORROPIA: A new thermodynamic equilibrium model for multiphase multicomponent inorganic aerosols [J]. Aquatic Geochemistry, 1998, 4(1): 123-152. doi: 10.1023/A:1009604003981

[23]

YANG B, ZHOU L L, XUE N D, et al. Source apportionment of polycyclic aromatic hydrocarbons in soils of Huanghuai Plain, China: Comparison of three receptor models [J]. Science of the Total Environment, 2013, 443: 31-39. doi: 10.1016/j.scitotenv.2012.10.094

[24]

衣雅男, 侯战方, 孟静静, 等. 聊城市冬季PM_2.5中水溶性化合物的昼夜变化特征及来源解析 [J]. 环境科学, 2019, 40(10): 4319-4329. YI Y N, HOU Z F, MENG J J, et al. Diurnal variations and source analysis of water-soluble compounds in PM_2.5 during the winter in Liaocheng city [J]. Environmental Science, 2019, 40(10): 4319-4329(in Chinese).

[25]

别淑君, 杨凌霄, 高颖, 等. 济南市背景区域大气PM_2.5污染特征及其对能见度的影响 [J]. 环境科学, 2019, 40(9): 3868-3874. BIE S J, YANG L X, GAO Y, et al. Characteristics of atmospheric PM_2.5 pollution and its influence on visibility in background areas of Ji'nan [J]. Environmental Science, 2019, 40(9): 3868-3874(in Chinese).

[26]

丁新航, 梁越, 肖化云, 等. 太原市采暖季清洁天与灰霾天PM_2.5中水溶性无机离子组成及来源分析 [J]. 环境化学, 2019, 38(6): 1356-1366. doi: 10.7524/j.issn.0254-6108.2018121102 DING X H, LIANG Y, XIAO H Y, et al. Composition and source analysis of water-soluble inorganic ions of PM_2.5 in clean and haze days during heating season in Taiyuan City [J]. Environmental Chemistry, 2019, 38(6): 1356-1366(in Chinese). doi: 10.7524/j.issn.0254-6108.2018121102

[27]

SHENG Z Z, CHE H Z, CHEN Q L, et al. Aerosol vertical distribution and optical properties of different pollution events in Beijing in autumn 2017 [J]. Atmospheric Research, 2019, 215: 193-207. doi: 10.1016/j.atmosres.2018.08.029

[28]

张颖龙, 李莉, 宋刘明, 等. 嘉善冬季PM_2.5化学组分特征及来源分析 [J]. 环境化学, 2021, 40(3): 754-764. doi: 10.7524/j.issn.0254-6108.2020062303 ZHANG Y L, LI L, SONG L M, et al. Chemical components characteristic and source apportionment of PM_2.5 during winter in Jiaxing [J]. Environmental Chemistry, 2021, 40(3): 754-764(in Chinese). doi: 10.7524/j.issn.0254-6108.2020062303

[29]

张婷, 曹军骥, 刘随心. 宝鸡市PM_2.5中水溶性离子组分污染特征及来源分析 [J]. 地球环境学报, 2017, 8(1): 46-54. doi: 10.7515/JEE201701006 ZHANG T, CAO J J, LIU S X. Pollution characteristics and sources of water-soluble ions in PM_2.5 in Baoji [J]. Journal of Earth Environment, 2017, 8(1): 46-54(in Chinese). doi: 10.7515/JEE201701006

[30]

宿文康, 鲍晓磊, 倪爽英, 等. 2018年石家庄市秋冬季典型霾污染特征 [J]. 环境科学, 2019, 40(11): 4755-4763. SU W K, BAO X L, NI S Y, et al. Characteristics of haze pollution episodes during autumn and winter in 2018 in Shijiazhuang [J]. Environmental Science, 2019, 40(11): 4755-4763(in Chinese).

[31]

张勇, 刘随心, 曹军骥, 等. 汉中市秋季PM_2.5昼夜变化特征 [J]. 地球环境学报, 2019, 10(1): 79-86. ZHANG Y, LIU S X, CAO J J, et al. Diurnal variation characteristics of PM_2.5 in Hanzhong in autumn [J]. Journal of Earth Environment, 2019, 10(1): 79-86(in Chinese).

[32]

李欢, 唐贵谦, 张军科, 等. 2017—2018年北京大气PM_2.5中水溶性无机离子特征 [J]. 环境科学, 2020, 41(10): 4364-4373. LI H, TANG G Q, ZHANG J K, et al. Characteristics of water-soluble inorganic ions in PM_2.5 in Beijing during 2017-2018 [J]. Environmental Science, 2020, 41(10): 4364-4373(in Chinese).

[33]

杨留明, 王申博, 郝祺, 等. 郑州市PM_2.5中水溶性离子特征及来源分析 [J]. 环境科学, 2019, 40(7): 2977-2984. YANG L M, WANG S B, HAO Q, et al. Characteristics and source analysis of water-soluble ions in PM_2.5 in Zhengzhou [J]. Environmental Science, 2019, 40(7): 2977-2984(in Chinese).

[34]

WANG Y, ZHUANG G S, TANG A H, et al. The ion chemistry and the source of PM_2.5 aerosol in Beijing [J]. Atmospheric Environment, 2005, 39(21): 3771-3784. doi: 10.1016/j.atmosenv.2005.03.013

[35]

李欣悦, 张凯山, 武文琪, 等. 成都市城区大气细颗粒物水溶性离子污染特征 [J]. 中国环境科学, 2021, 41(1): 91-101. doi: 10.3969/j.issn.1000-6923.2021.01.011 LI X Y, ZHANG K S, WU W Q, et al. Characterization of water-soluble ions pollution of atmospheric fine particles in Chengdu City [J]. China Environmental Science, 2021, 41(1): 91-101(in Chinese). doi: 10.3969/j.issn.1000-6923.2021.01.011

[36]

宿文康, 鲍晓磊, 孟琛琛, 等. 冬季PM_2.5中无机水溶性离子与大气相对湿度的相关性 [J]. 环境科学学报, 2021, 41(5): 1734-1740. SU W K, BAO X L, MENG C C, et al. Correlation analysis on inorganic water soluble ions in PM_2.5 and relative humidity of atmosphere in winter [J]. Acta Scientiae Circumstantiae, 2021, 41(5): 1734-1740(in Chinese).

[37]

BAUER S E, KOCH D, UNGER N, et al. Nitrate aerosols today and in 2030: A global simulation including aerosols and tropospheric ozone [J]. Atmospheric Chemistry and Physics, 2007, 7(19): 5043-5059. doi: 10.5194/acp-7-5043-2007

[38]

宝鸡市统计局. 2012年宝鸡市国民经济和社会发展统计公报[EB/OL]. [2013-3-18]. http://tjj.baoji.gov.cn/art/2013/3/18/art_1959_182233.html.

[39]

宝鸡市统计局. 2019年宝鸡市国民经济和社会发展统计公报[EB/OL]. [2021-12-6]. http://tjj.baoji.gov.cn/art/2020/4/1/art_1959_533131.html

[40]

XU L L, CHEN X Q, CHEN J S, et al. Seasonal variations and chemical compositions of PM_2.5 aerosol in the urban area of Fuzhou, China [J]. Atmospheric Research, 2012, 104/105: 264-272. doi: 10.1016/j.atmosres.2011.10.017

[41]

YANG Y J, ZHOU R, YU Y, et al. Size-resolved aerosol water-soluble ions at a regional background station of Beijing, Tianjin, and Hebei, North China [J]. Journal of Environmental Sciences, 2017, 55: 146-156. doi: 10.1016/j.jes.2016.07.012

[42]

PATHAK R K, LOUIE P K K, CHAN C K. Characteristics of aerosol acidity in Hong Kong [J]. Atmospheric Environment, 2004, 38(19): 2965-2974. doi: 10.1016/j.atmosenv.2004.02.044

[43]

HUA Y, CHENG Z, WANG S X, et al. Characteristics and source apportionment of PM_2.5 during a fall heavy haze episode in the Yangtze River Delta of China [J]. Atmospheric Environment, 2015, 123: 380-391. doi: 10.1016/j.atmosenv.2015.03.046

[44]

吴丹, 蔺少龙, 杨焕强, 等. 杭州市PM_2.5中水溶性离子的污染特征及其消光贡献 [J]. 环境科学, 2017, 38(7): 2656-2666. WU D, LIN S L, YANG H Q, et al. Pollution characteristics and light extinction contribution of water-soluble ions of PM_2.5 in Hangzhou [J]. Environmental Science, 2017, 38(7): 2656-2666(in Chinese).

[45]

XU L L, DUAN F K, HE K B, et al. Characteristics of the secondary water-soluble ions in a typical autumn haze in Beijing [J]. Environmental Pollution, 2017, 227: 296-305. doi: 10.1016/j.envpol.2017.04.076