废弃塑料处置地典型植物多溴二苯醚污染特征

金璐, 唐阵武, 张连振, 何洁, 陶义. 废弃塑料处置地典型植物多溴二苯醚污染特征[J]. 环境化学, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
引用本文: 金璐, 唐阵武, 张连振, 何洁, 陶义. 废弃塑料处置地典型植物多溴二苯醚污染特征[J]. 环境化学, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
JIN Lu, TANG Zhenwu, ZHANG Lianzhen, HE Jie, TAO Yi. Polybrominated diphenyl ethersin in plants from a plastic waste recycling area in China[J]. Environmental Chemistry, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
Citation: JIN Lu, TANG Zhenwu, ZHANG Lianzhen, HE Jie, TAO Yi. Polybrominated diphenyl ethersin in plants from a plastic waste recycling area in China[J]. Environmental Chemistry, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008

废弃塑料处置地典型植物多溴二苯醚污染特征

  • 基金项目:

    国家环境保护公益性行业科研专项(201009026-02,201309023);国家自然科学基金项目(41001329)资助.

Polybrominated diphenyl ethersin in plants from a plastic waste recycling area in China

  • Fund Project:
  • 摘要: 为了解土壤高污染的废弃塑料处置地植物体多溴二苯醚(PBDEs)累积水平,对废弃塑料处置地13种典型植物中21种多溴二苯醚的浓度水平、组成和污染特征进行了研究.结果表明,该区域植物中∑PBDEs含量为11.3—122 ng·g-1,平均为51.2 ng·g-1,与我国电子废物处置地植物体污染水平相似,远高于一般区域植物体PBDEs污染水平.不同植物体内PBDEs的含量差异较大,其中牵牛花中PBDEs的含量最高,牛筋草中PBDEs含量最低.废弃塑料处置地植物体中BDE 209的含量为10.8—116 ng·g-1,为最主要的PBDEs同系物单体,平均占∑PBDEs的96.9%以上.其余单体中,以BDE 47和BDE 208等含量相对较高,但占总PBDEs总含量均不到1%.废弃塑料处置地植物体较电子废物处置地和一般区域植物体表现出更明显的十溴二苯醚污染特征.
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  • [1] Jiang J, Shi S, Chen T. Occurrence of polybrominated diphenyl ethers in fish and shell fish downstream from electronic-waste recycling plants[J]. J Environ Sci (China), 2010, 22(5):723-730
    [2] 张利飞, 黄业茹, 董亮. 多溴联苯醚在中国的污染现状研究进展[J]. 环境化学, 2010, 29(5): 787-795
    [3] de Wit C A. An overview of brominated flame retardants in the environment[J]. Chemosphere, 2002, 46(5): 583-624
    [4] Rahman F, Langford K H, Scrimshaw M D, et al. Polybrominated diphenyl ether (PBDE) flame retardants[J]. Sci Total Environ, 2001, 275(1/3): 1-17
    [5] Leung A O, Luksemburg W J, Wong A S, et al. Spatial distribution of polybrominated diphenyl ethers and polychlorinated dibenzo-p-dioxins and dibenzofurans in soil and combusted residue at Guiyu, an electronic waste recycling site in southeast China[J]. Environ Sci Technol, 2007, 41(8): 2730-2737
    [6] Mueller K E, Mueller-Spitz S R, Henry H F, et al. Fate of pentabrominated diphenyl ethers in soil: abiotic sorption, plant uptake, and the impact of interspecific plant interactions[J]. Environ Sci Technol, 2006, 40(21):6662-6667
    [7] Huang H, Zhang S, Christie P, et al. Behavior of decabromodiphenyl ether (BDE-209) in the soil-plant system: uptake, translocation and metabolism in plants and dissipation in soil[J]. Environ Sci Technol, 2010, 44(2):663-667
    [8] Wang Y, Luo C, Li J, et al. Characterization of PBDEs in soils and vegetations near an e-waste recycling site in South China[J]. Environ Pollut, 2011, 159(10):2443-2448
    [9] Tanabe S. PBDEs, an emerging group of persistent pollutants[J]. Mar Pollut Bull, 2004, 49(5/6): 369-370
    [10] 陆少游, 龚诗涵, 袁晶, 等. 我国某塑料垃圾拆解地周边居民多环芳烃内暴露水平调查[J]. 环境化学, 2012, 31(5): 593-598
    [11] 曾甯, 姚建, 唐阵武, 等. 典型废旧塑料处置地土壤中多溴联苯醚污染特征[J]. 环境科学研究, 2013, 26(4): 432-438
    [12] 傅海辉, 黄启飞, 孟昭福, 等.加速溶剂萃取-气质联用同步测定土壤中17组分多溴二苯醚[J]. 环境科学研究, 2012, 25(5): 595-604
    [13] Yu Y X, Huang N B, Zhang X Y, et al. Polybrominated diphenyl ethers in food and associated human daily intake assessment considering bioaccessibility measured by simulated gastrointestinal digestion[J]. Chemosphere, 2011, 83(2): 152-160
    [14] Jin J, Liu W, Wang Y, et al. Levels and distribution of polybrominated diphenyl ethers in plant, shellfish and sediment samples from Laizhou Bay in China[J]. Chemosphere, 2008, 71(6):1043-1050
    [15] Tian M, Chen S J, Wang J, et al. Plant uptake of atmospheric brominated flame retardants at an E-waste site in southern China[J]. Environ Sci Technol, 2012, 46 (5):2708-2714
    [16] Qin P H, Ni H G, Liu Y S, et al. Occurrence, distribution, and source of polybrominated diphenyl ethers in soil and leaves from Shenzhen Special Economic Zone, China[J]. Environ Monit Assess, 2011, 174(1/4):259-270
    [17] Zhao G, Zhou H, Wang D, et al. PBBs, PBDEs, and PCBs in foods collected from e-waste disassembly sites and daily intake by local residents[J]. Sci Total Environ, 2009, 407(8): 2565-2575
    [18] St-Amand A D, Mayer P M, Blais J M, et al. Seasonal trends in vegetation and atmospheric concentrations of PAHs and PBDEs near a sanitary landfill[J]. Atmos Environ, 2008, 42(13): 2948-2958
    [19] Parolini M, Guazzoni N, Binelli A, et al. Polybrominated diphenyl ether contamination in soil, vegetation, and cow milk from a high-mountain pasture in the Italian Alps[J]. Arch Environ Contam Toxicol, 2012, 63(1):29-44
    [20] 高永飞, 王璞, 陈卫海, 等. 喜马拉雅山区葇籽草和棘豆样品中PCBs、PBDEs和PCDD/Fs的分析[J]. 环境化学, 2012, 31(1): 26-30
    [21] Yang Z Z, Zhao X R, Zhao Q, et al. Polybrominated diphenyl ethers in leaves and soil from typical electronic waste polluted area in South China[J]. Bull Environ Contam Toxicol, 2008, 80(4):340-344
    [22] Hardy M L. The toxicology of the three commercial polybrominated diphenyl oxide (ether) flame retardants[J]. Chemosphere, 2002, 46(5): 757-777
    [23] Alaee M, Arias P, Sjödin A, et al. An overview of commercially used brominated flame retardants, their applications, their use patterns in different countries/regions and possible modes of release[J]. Environ Int, 2003, 29(6): 683-689
    [24] Darnerud P O, Eriksen G S, Jóhannesson T, et al. Polybrominated diphenyl ethers: occurrence, dietary exposure, and toxicology[J]. Environ Health Perspect, 2001, 109(1): 49-68
    [25] LaA Guardia M J, Hale R C, Harvey E. Detailed polybrominated diphenyl ether (PBDE) congener composition of the widely used penta-, octa-, and deca-PBDE technical flame-retardant mixtures[J]. Environ Sci Technol, 2006, 40(20): 6247-6254
    [26] Behnisch P A, Hosoe K, Sakai S. Brominated dioxin-like compounds: in vitro assessment in comparison to classical dioxin-like compounds and other polyaromatic compounds[J]. Environ Int, 2003, 29(6):861-877
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  • 收稿日期:  2013-09-20
金璐, 唐阵武, 张连振, 何洁, 陶义. 废弃塑料处置地典型植物多溴二苯醚污染特征[J]. 环境化学, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
引用本文: 金璐, 唐阵武, 张连振, 何洁, 陶义. 废弃塑料处置地典型植物多溴二苯醚污染特征[J]. 环境化学, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
JIN Lu, TANG Zhenwu, ZHANG Lianzhen, HE Jie, TAO Yi. Polybrominated diphenyl ethersin in plants from a plastic waste recycling area in China[J]. Environmental Chemistry, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008
Citation: JIN Lu, TANG Zhenwu, ZHANG Lianzhen, HE Jie, TAO Yi. Polybrominated diphenyl ethersin in plants from a plastic waste recycling area in China[J]. Environmental Chemistry, 2014, 33(6): 901-907. doi: 10.7524/j.issn.0254-6108.2014.06.008

废弃塑料处置地典型植物多溴二苯醚污染特征

  • 1.  华北电力大学资源与环境研究院, 北京, 102206;
  • 2.  中国环境科学研究院, 北京, 100012
基金项目:

国家环境保护公益性行业科研专项(201009026-02,201309023);国家自然科学基金项目(41001329)资助.

摘要: 为了解土壤高污染的废弃塑料处置地植物体多溴二苯醚(PBDEs)累积水平,对废弃塑料处置地13种典型植物中21种多溴二苯醚的浓度水平、组成和污染特征进行了研究.结果表明,该区域植物中∑PBDEs含量为11.3—122 ng·g-1,平均为51.2 ng·g-1,与我国电子废物处置地植物体污染水平相似,远高于一般区域植物体PBDEs污染水平.不同植物体内PBDEs的含量差异较大,其中牵牛花中PBDEs的含量最高,牛筋草中PBDEs含量最低.废弃塑料处置地植物体中BDE 209的含量为10.8—116 ng·g-1,为最主要的PBDEs同系物单体,平均占∑PBDEs的96.9%以上.其余单体中,以BDE 47和BDE 208等含量相对较高,但占总PBDEs总含量均不到1%.废弃塑料处置地植物体较电子废物处置地和一般区域植物体表现出更明显的十溴二苯醚污染特征.

English Abstract

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