地下水药物的赋存、源解析及运移机理

林双双, 张亚雷, 石璐, 周雪飞. 地下水药物的赋存、源解析及运移机理[J]. 环境化学, 2012, 31(12): 1849-1854.
引用本文: 林双双, 张亚雷, 石璐, 周雪飞. 地下水药物的赋存、源解析及运移机理[J]. 环境化学, 2012, 31(12): 1849-1854.
LIN Shuangshuang, ZHANG Yalei, SHI Lu, ZHOU Xuefei. Occurrence, sources and migration mechanism of pharmaceuticals in groundwater[J]. Environmental Chemistry, 2012, 31(12): 1849-1854.
Citation: LIN Shuangshuang, ZHANG Yalei, SHI Lu, ZHOU Xuefei. Occurrence, sources and migration mechanism of pharmaceuticals in groundwater[J]. Environmental Chemistry, 2012, 31(12): 1849-1854.

地下水药物的赋存、源解析及运移机理

  • 基金项目:

    国家自然科学基金(41072172)

    污染控制与资源化研究国家重点实验室自主课题(PCRRY11015,PCRRY11004)

    中国博士后基金资助项目(20100480625)

    中国博士后基金特别资助项目(201104274)资助.

Occurrence, sources and migration mechanism of pharmaceuticals in groundwater

  • Fund Project:
  • 摘要: 近年来,大量使用的医用和兽用药物可通过人体或动物的排泄、不合理的弃置等直接或间接途径迁移到地下水体中.残留在地下水中的药物经过长时间的富集,可能对水环境系统及人类的健康产生许多负面效应.为全面了解地下水中药物的污染现状并及时防治其对地下水的进一步污染,本文综述了地下水药物的赋存现状及其主要来源途径,总结了药物在地下的运移机理及其主要的影响因素.
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  • [1] Watanabe N, Harter T H, Bergamaschi B A. Environmental occurrence and shallow ground water detection of the antibiotic monensin from dairy farms[J]. Journal of Environmental Quality, 2008, 37(5): S78-S85
    [2] Lapworth D J, Baran N, Stuart M E, et al.Emerging organic contaminants in groundwater: A review of sources, fate and occurrence[J]. Environmental Pollution, 2012, 163: 287-303
    [3] Carrara C, Ptacek C J, Robertson W D, et al. Fate of pharmaceutical and trace organic compounds in three septic system plumes, Ontario, Canada[J]. Environmental Science & Technology, 2008, 42(8): 2805-2811
    [4] Sacher F, Lange F T, Brauch H J, et al. Pharmaceuticals in groundwaters-analytical methods and results of a monitoring program in Baden-Württemberg, Germany[J]. Journal of Chromatography A,2001, 938(1/2): 199-210
    [5] Buerge I J, Buser H R, Kahle M, et al. Ubiquitous occurrence of the artificial sweetener acesulfame in the aquatic environment: An ideal chemical marker of domestic wastewater in groundwater[J]. Environmental Science & Technology, 2009, 43(12): 4381-4385
    [6] Bruchet A, Hochereau C, Picard C, et al. Analysis of drugs and personal care products in French source and drinking waters: The analytical challenge and examples of application[J]. Water Science & Technology, 2004, 52(8): 53-61
    [7] Batt A L, Snow D D, Aga D S. Occurrence of sulfonamide antimicrobials in private wells in Washington County, Idaho, USA[J]. Chemosphere,2006, 64(11): 1963-1971
    [8] Diaz-Cruz M S, Garcia-Galan M J, Barcel D. Highly sensitive simultaneous determination of sulfonamide antibiotics and one metabolite in environmental samples by liquid chromatography-quadrupole linear ion trap-mass spectrometry[J]. Chromatogr A, 2008, 1193(1/2): 50-59
    [9] Holm J V, Rugge K, Bjerg P L, et al. Occurrence and distribution of pharmaceutical organic compounds in the groundwater downgradient of a landfill (Grindsted, Denmark)[J]. Environmental Science & Technology, 1995, 29(5): 1415-1420
    [10] 洪蕾洁,石璐,张亚雷,等. 固相萃取-高效液相色谱法同时测定水体中的10种磺胺类抗生素[J]. 环境科学, 2012, 33(2):652-657
    [11] Vulliet E, Cren-Olivé C. Screening of pharmaceuticals and hormones at the regional scale, in surface and groundwaters intended to human consumption[J]. Environmental Pollution, 2011, 159(10): 2929-2934
    [12] Barnes K K, Kolpin D W, Furlong E T, et al. A national reconnaissance of pharmaceuticals and other organic wastewater contaminants in the United States- I)Groundwater[J]. Science of the Total Environment, 2008, 402(2/3):192-200
    [13] Heberer T. Tracking persistent pharmaceutical residues from municipal sewage to drinking water[J]. Journal of Hydrology, 2002, 266(3/4): 175-189
    [14] Loos R, Locoro G, Comero S, et al. Pan-European survey on the occurrence of selected polar organic persistent pollutants in ground water[J]. Water Research, 2010, 44(14): 4115-4126
    [15] Drewes J E, Heberer T, Rauch T, et al. Fate of pharmaceuticals during ground water recharge[J]. Ground Water Monitoring and Remediation, 2003, 23(3): 64-72
    [16] Heberer T, Mechlinski A, Fanck B, et al. Field studies on the fate and transport of pharmaceutical residues in bank filtration[J]. Ground Water Monitoring and Remediation, 2004, 24(2): 70-77
    [17] Fram M S, Belitz K. Occurrence and concentrations of pharmaceutical compounds in groundwater used for public drinking-water supply in California[J]. Science of the Total Environment, 2011, 409(18): 3049-3417
    [18] Glassmeyer S T, Furlong E T, Kolpin D W, et al. Transport of chemical and microbial contaminants from known wastewater discharges: Potential for use as indicators of human fecal contamination[J]. Environmental Science & Technology, 2005, 39(14): 5157-5169
    [19] Díaz-Cruz M S, BarcelóD. Trace organic chemicals contamination in ground water recharge[J]. Chemosphere, 2008, 72(3): 333-342
    [20] Eckel W P, Ross B, Isensee R K. Pentobarbital found in ground water-reply[J]. Ground Water, 1993, 31(5): 801-804
    [21] Bartelt-Hunt S, Snow D D, Damon-Powell T, et al. Occurrence of steroid hormones and antibiotic in shallow groundwater impacted by livestock waste control facilities[J]. Journal of Contaminant Hydrology, 2011, 123(3/4): 94-103
    [22] 周启星,罗义,王美娥. 抗生素的环境残留、生态毒性及抗性基因污染[J].生态毒理学报, 2007, 2(3):243-251
    [23] Hartmann A, Alder A C, Koller T, et al. Identification of fluoroquinolone antibiotics as the main source of umuC genotoxicity in native hospital wastewater[J]. Environmental Toxicology and Chemistry, 1998, 17(3): 377-382
    [24] Sarmah A K, Meyer M T, Boxall A B A. A global perspective on the use, sales, exposure pathways, occurrence, fate and effects of veterinary antibiotics (VAs) in the environment[J]. Chemosphere, 2006, 65(5): 725-759
    [25] Clarke B O, Smith S R. Review of 'emerging’ organic contaminants in biosolids and assessment of international research priorities for the agricultural use of biosolids[J]. Environment International, 2011, 37(1): 226-247
    [26] Lewandowski J, Putschew A, Schwesig D, et al. Fate of organic micropollutants in the hyporheic zone of a eutrophic lowland stream: results of a preliminary field study[J]. Science of the Total Environment, 2011, 409(10):1824-1835
    [27] Ellis J B. Pharmaceutical and personal care products (PPCPs) in urban receiving waters[J]. Environmental Pollution,2006, 144(1): 184-189
    [28] Snyder S A, Leising J, Westerhoff P, et al. Biological and physical attenuation of endocrine disruptors and pharmaceuticals: Implications for water reuse[J]. Ground Water Monitoring and Remediation, 2004, 24(2): 108-118
    [29] Laws B V, Dickenson E R V, Johnson T A, et al. Attenuation of contaminants of emerging concern during surface-spreading aquifer recharge[J]. Science of the Total Environment, 2011, 409(6): 1087-1094
    [30] Tolls J. Sorption of veterinary pharmaceuticals in soils: a review[J]. Environmental Science & Technology, 2001, 35(17): 3397-3406
    [31] Watanabe N, Bergamaschi B A, Loftin K A, et al. Use and environmental occurrence of antibiotics in freestall dairy farms with manure forage fields[J]. Environmental Science & Technology, 2010, 44(17): 6591-6600
    [32] Shinohara H, Murakami M, Managaki S, et al. Removal of water-soluble organic micro-pollutants by soil infiltration[J]. Journal of Environmental Science, 2006, 19(5): 435-444
    [33] Scheytt T, Mersmann P, Lindstädt R, et al. Determination of sorption coefficients of pharmaceutically active substances carbamazepine, diclofenac, and ibuprofen, in sandy sediments[J]. Chemosphere, 2005, 60(2): 245-253
    [34] Semple K T, Doick K J, Wick L Y, et al. Microbial interactions with organic contaminants in soil: Definitions, processes and measurement[J]. Environmental Pollution, 2007, 150(1): 166-176
    [35] Johnson A C, Hughes C D, Williams R J, et al. Potential for aerobic isoproturon biodegradation and sorption in the unsaturated and saturated zones of a chalk aquifer[J]. Journal of Contaminant Hydrology, 1998, 30(3/4): 281-297
    [36] 张从良,王岩,壬福安. 磺胺类药物在土壤中的微生物降解[J].农业环境科学学报, 2007, 26(5):1658-1662
    [37] Benotti M J, Bronawell B J. Microbial degradation of pharmaceuticals in estuarine and coastal seawater[J]. Environmental Pollution, 2009, 157(3): 994-1002
    [38] Thiele-Bruhn S, Peters D. Photodegradation of pharmaceutical antibiotics on slurry and soil surfaces[J]. Landbauforschung Volkenrode, 2007,57:13-23
    [39] Loftin K A, Adams C D, Meyer M T, et al. Effects of ionic strength, temperature, and pH on degradation of selected antibiotics[J]. Journal of Environmental Quality, 2008, 37(2): 378-386
    [40] Katz B G, Griffin D W, Davis J H. Groundwater quality impacts from land application of treated municipal wastewater in a large karstic spring basin: Chemical and micbiological indicators[J]. Science of the Total Environment,2009, 407(8):2872-2886
    [41] Chefetz B, Mualem T, Ben-Ari J. Sorption and mobility of pharmaceutical compounds in soil irrigated with reclaimed wastewater[J]. Chemosphere, 2008, 73(8): 1335-1343
    [42] 文春波,张从良,王岩. 磺胺嘧啶在土壤中的降解与迁移研究[J].农业环境科学学报,2007, 26(5):1677-1680
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出版历程
  • 收稿日期:  2012-01-01
林双双, 张亚雷, 石璐, 周雪飞. 地下水药物的赋存、源解析及运移机理[J]. 环境化学, 2012, 31(12): 1849-1854.
引用本文: 林双双, 张亚雷, 石璐, 周雪飞. 地下水药物的赋存、源解析及运移机理[J]. 环境化学, 2012, 31(12): 1849-1854.
LIN Shuangshuang, ZHANG Yalei, SHI Lu, ZHOU Xuefei. Occurrence, sources and migration mechanism of pharmaceuticals in groundwater[J]. Environmental Chemistry, 2012, 31(12): 1849-1854.
Citation: LIN Shuangshuang, ZHANG Yalei, SHI Lu, ZHOU Xuefei. Occurrence, sources and migration mechanism of pharmaceuticals in groundwater[J]. Environmental Chemistry, 2012, 31(12): 1849-1854.

地下水药物的赋存、源解析及运移机理

  • 1.  同济大学长江水环境教育部重点实验室, 上海, 200092;
  • 2.  同济大学污染控制与资源化研究国家重点实验室, 上海, 200092
基金项目:

国家自然科学基金(41072172)

污染控制与资源化研究国家重点实验室自主课题(PCRRY11015,PCRRY11004)

中国博士后基金资助项目(20100480625)

中国博士后基金特别资助项目(201104274)资助.

摘要: 近年来,大量使用的医用和兽用药物可通过人体或动物的排泄、不合理的弃置等直接或间接途径迁移到地下水体中.残留在地下水中的药物经过长时间的富集,可能对水环境系统及人类的健康产生许多负面效应.为全面了解地下水中药物的污染现状并及时防治其对地下水的进一步污染,本文综述了地下水药物的赋存现状及其主要来源途径,总结了药物在地下的运移机理及其主要的影响因素.

English Abstract

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